New insight into unconventional superconductivity
The kagome pattern, a network of corner-sharing triangles, is well known amongst traditional Japanese basket weavers — and condensed matter physicists. The unusual geometry of metal atoms in the kagome lattice and resulting electron behaviour makes it a playground for probing weird and wonderful quantum phenomena that form the basis of next-generation device research.
A key example is unconventional — such as high-temperature — superconductivity, which does not follow the conventional laws of superconductivity. Most superconducting materials exhibit their seemingly magical property of zero resistance at a few degrees Kelvin: temperatures that are simply impractical for most applications. Materials that exhibit so-called ‘high-temperature’ superconductivity, at temperatures achievable with liquid nitrogen cooling (or even at room temperature), are a tantalising prospect. Finding and synthesising new materials that exhibit unconventional superconductivity has become the condensed matter physicist’s Holy Grail — but getting there involves a deeper understanding ofexotic, topological electronic behaviour in materials.
An exotic type of electron transport behaviour that results in a spontaneous flow of charge in loops has long been debated as a precursor to high-temperature superconductivity and as a mechanism behind another mysterious phenomenon: the quantum anomalous Hall effect. This topological effect, the subject of F. Duncan M. Haldane’s 2016 Nobel Prize winning work, occurs in certain two-dimensional electronic materials and relates to the generation of a current even in the absence of an applied magnetic field. Understanding the quantum anomalous Hall effect is important not only for fundamental physics, but also for the potential applications in novel electronics and devices. Now, a PSI-led international collaboration has discovered strong evidence supporting this elusive electron transport behaviour.
Time-reversal symmetry-breaking charge ordering in the kagome superconductor KV3Sb5
The team, led by researchers from PSI’s Laboratory for Muon Spin Spectroscopy, discovered weak internal magnetic fields indicative of an exotic charge ordering in a correlated kagome superconductor. These magnetic fields break so-called time-reversal symmetry, a type of symmetry that means that the laws of physics are the same whether you look at a system going forward or backward in time.
A natural explanation of the occurrence of time-reversal symmetry-breaking fields is a novel type of charge order. The charge ordering can be understood as a periodic modulation of the electron density through the lattice and rearrangement of the atoms into a higher-order (superlattice) structure. The team focused their study on the kagome lattice, KV3Sb5, which superconducts below 2.5 Kelvin. Below a higher critical temperature of approximately 80 Kelvin, a giant quantum anomalous Hall effect is observed in the material, which was previously unexplained. The exotic charge ordering appears below this critical temperature of approximately 80 Kelvin, termed the ‘charge ordering temperature’. More