Uncovering unexpected properties in a complex quantum material
A new study describes previously unexpected properties in a complex quantum material known as Ta2NiSe5. Using a novel technique developed at Penn, these findings have implications for developing future quantum devices and applications. This research, published in Science Advances, was conducted by University of Pennsylvania graduate student Harshvardhan Jogand led by professor Ritesh Agarwal in collaboration with professor Eugene Mele and Luminita Harnagea from the Indian Institute of Science Education and Research.
While the field of quantum information science has experienced progress in recent years, the widespread use of quantum computers is still limited. One challenge is the ability to only use a small number of “qubits,” the unit that performs calculations in a quantum computer, because current platforms are not designed to allow multiple qubits to “talk” to one another. In order to address this challenge, materials need to be efficient at quantum entanglement, which occurs when the states of qubits remain linked no matter their distance from one another, as well as coherence, or when a system can maintain this entanglement.
In this study, Jog looked at Ta2NiSe5, a material system that has strong electronic correlation, making it attractive for quantum devices. Strong electronic correlation means that the material’s atomic structure is linked to its electronic properties and the strong interaction that occurs between electrons.
To study Ta2NiSe5, Jog used a modification of a technique developed in the Agarwal lab known as the circular photogalvanic effect, where light is engineered to carry an electric field and is able to probe different material properties. Developed and iterated in the past several years, this technique has revealed insights about materials such as silicon and Weyl semimetals in ways that are not possible with conventional physics and materials science experiments.
But the challenge in this study, says Agarwal, is that this method has only been applied in materials without inversion symmetry, whereas Ta2NiSe5 does haveinversion symmetry, Jog “wanted to see if this technique can be used to study materials which have inversion symmetry which, from a conventional sense, should not be producing this response,” says Agarwal.
After connecting with Harnagea to obtain high-quality samples of Ta2NiSe5, Jog and Agarwal used a modified version of the circular photogalvanic effect and were surprised to see that there was a signal being produced. After conducting additional studies to ensure that this was not an error or an experimental artifact, they worked with Mele to develop a theory that could help explain these unexpected results. More